BUSCADOR RECOLECTA

HRTEM image of a thick walled TbS-CrS2 nanotubular structure, elemental quantification of a radial EELS line highlighting the O-T alternating system and the surface oxidation of one wavy NT, EELS analyses of the surface of one nanotube highlighting the CrS termination, and Cs-HRTEM micrograph of the surface of a TbS-CrS2 nanotube showing the presence of an outer crystalline layer., Peer reviewed

By combining ab initio simulations with state-of-the-art electron microscopy and electron energy loss spectroscopy, we study the mechanism of electron beam damage in nitrogen-doped graphene and carbon nanotubes. Our results show that the incorporation of nitrogen atoms results in noticeable knock-on damage in these structures already at an acceleration voltage of 80 kV, at which essentially no damage is created in pristine structures at corresponding doses. Contrary to an early estimate predicting rapid destruction via sputtering of the nitrogen atoms, in the case of substitutional doping, damage is initiated by displacement of carbon atoms neighboring the nitrogen dopant, leading to the conversion of substitutional dopant sites into pyridinic ones. Although such events are relatively rare at 80 kV, they become significant at higher voltages typically used in electron energy loss spectroscopy studies. Correspondingly, we measured an energy loss spectrum time series at 100 kV that provides direct evidence for such conversions in nitrogen-doped single-walled carbon nanotubes, in excellent agreement with our theoretical prediction. Besides providing an improved understanding of the irradiation stability of these structures, we show that structural changes cannot be neglected in their characterization employing high-energy electrons., T.S. received support from the Finnish Foundation for Technology Promotion. T.S., H.J., and E.I.K. further acknowledge financial support from the CNB-E project of the Aalto MIDE program and from the LiBaCAM project of TEKES. J.K. and A.V.K. acknowledge financial support from Helsinki University Funds and Academy of Finland through several projects as well as CSC Ltd. Finland for computational resources. S.K., U.K., and J.C.M. acknowledge the financial support by the DFG (German Research Foundation) and the Ministry of Science, Research and the Arts (MWK) of Baden-Wuerttemberg in the frame of the SALVE (Sub Angstrom Low-Voltage Electron microscopy) project. V.S. acknowledges an EC Grant No. 266391 related to the project ELECTROGRAPH (FP7/2007-2013)., Peer reviewed

Supplementary Figure S1: Temperature and relative humidity values recorded during the summer2020 and summer2021 greenhouse trials. Supplementary Figure S2: Water evaporation rate assessed in chamber-controlled conditions. Supplementary Figure S3: Vegetative traits assessed during the summer2020 greenhouse trial before stress treatment initiation. Supplementary Figure S4: Stem thickness values assessed during the summer2020 and summer2021 greenhouse trials. Supplementary Figure S5: General overview of TILLING and EcoTILLING analyses. Supplementary Table S1: Natural germplasm collection screened for heat and drought stress tolerance under nursery greenhouse conditions. Supplementary Table S2: Primers used for the HRM analysis of the SlCBL10 gene. Supplementary Table S3: Tolerant M2 families identified during the screening of the EMS mutant collection under combined heat and drought stresses at nursery greenhouse conditions. Supplementary Table S4: Tolerant accessions identified during the screening of the natural germplasm collection under combined heat and drought stresses at nursery conditions. Supplementary Table S5: Phenotype traits evaluated during the summer2020 trial under combined heat and drought stresses. Mean ± standard deviations are included for plant height, stem thickness, and fruit setting. Supplementary Table S6: Phenotype traits evaluated during the summer2021 trial under combined heat and drought stresses. Mean ± standard deviations are included for plant height, stem thickness, and fruit setting. Supplementary Table S7. Single nucleotide variants of the SlCBL10 gene were detected in the EMS and the natural germplasm collections., Peer reviewed

The dataset includes the numerical data presented in Phys. Rev. X 14, 021017 (2024), "Unified treatment of light emission by inelastic tunneling: interaction of electrons and photons beyond the gap", written by Unai Muniain, Ruben Esteban, Javier Aizpurua and Jean-Jacques Greffet (doi.org/10.1103/PhysRevX.14.021017). The dataset is organized into folders according to the explanation in the README file., Agence Nationale de la Recherche (ANR-22-CE24-0011); MCIN/AEI/10.13039/501100011033 and “ERDF A way of making Europe" (Grants No. PID2019–107432 GB-I00 and No. PID2022-139579NB-I00); Basque Government (Project No. IT 1526-22 for consolidated groups of the Basque University), Peer reviewed

Figure S1 including the antibacterial effects of Au-CS nanocomposites against E. coli and S. aureus alone., Peer reviewed

Table S1: Primers, probes, (RT)-qPCR conditions, limit of quantification (LoQ/L) and limit of detection (LoD/L) for all targeted viruses included in this work. Table S2: Mengovirus recovery (%) and mean concentration values (Log10 gc/L) obtained by (RT)-qPCR of enteric viruses, crAssphage, and somatic coliphages (Log10 pfu/L). Table S3: Removal of enteric viruses between influent wastewater and reclaimed water (n = 9) by (RT)-qPCR. Table S4: Cycle threshold (Ct) values for the PMAxx-RT-qPCR optimization tests in influent wastewater samples. Table S5: Ct values by PMAxx-RT-qPCR for intact capsid enteric viruses and crAssphage in influent wastewater and reclaimed water. Table S6: Removal of enteric viruses in reclaimed water compared to influent wastewater (n = 9) by RT-qPCR and PMAxx-RT-qPCR., Peer reviewed

Table S1: Matrix of the factorial design adopted in the present study. Table S2: Experimental results obtained from the factorial design of experiments for the biochar yield and the response variables related to the carbon sequestration potential (xFC, molar H:C ratio, molar O:C ratio, R50 index, and “stable C”). Table S3: Experimental results for the yield of gas (ygas), yield of produced water (ywater), yield of condensable organic fraction (yorg), and cumulative yields of the main gaseous species (CO2, CO, CH4 and H2)., Peer reviewed

-NMR for 4 and Pro-PTX, Figures S1–S8 (PDF) -Movie S1: Preparation of Pd Alginate (MP4) -Molecular formula strings (CSV), Peer reviewed

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